:Dibenzothiophene

{{Chembox

| Watchedfields = changed

| verifiedrevid = 443634616

| Name = Dibenzothiophene

| ImageFile = Dibenzothiophen - Dibenzothiophene.svg

| ImageSize = 190px

| ImageAlt = Skeletal formula of dibenzothiophene

| ImageFile1 = Dibenzothiophene 3D ball.png

| ImageSize1 = 220px

| ImageAlt1 = Ball-and-stick model of the dibenzothiophene molecule

| ImageFile2 = DBTsample.jpg

| ImageSize2 = 180px

| ImageAlt2 = Sample

| PIN = Dibenzo[b,d]thiophene

| OtherNames = Diphenylene sulfide, DBT

| Section1 = {{Chembox Identifiers

| ChEBI_Ref = {{ebicite|correct|EBI}}

| ChEBI = 23681

| SMILES = c1ccc2c(c1)c3ccccc3s2

| ChemSpiderID_Ref = {{chemspidercite|correct|chemspider}}

| ChemSpiderID = 2915

| UNII_Ref = {{fdacite|correct|FDA}}

| UNII = Z3D4AJ1R48

| KEGG_Ref = {{keggcite|correct|kegg}}

| KEGG = D03777

| InChI = 1/C12H8S/c1-3-7-11-9(5-1)10-6-2-4-8-12(10)13-11/h1-8H

| InChIKey = IYYZUPMFVPLQIF-UHFFFAOYAY

| ChEMBL_Ref = {{ebicite|correct|EBI}}

| ChEMBL = 219828

| StdInChI_Ref = {{stdinchicite|correct|chemspider}}

| StdInChI = 1S/C12H8S/c1-3-7-11-9(5-1)10-6-2-4-8-12(10)13-11/h1-8H

| StdInChIKey_Ref = {{stdinchicite|correct|chemspider}}

| StdInChIKey = IYYZUPMFVPLQIF-UHFFFAOYSA-N

| CASNo_Ref = {{cascite|correct|CAS}}

| CASNo = 132-65-0

| RTECS = HQ3490550

| PubChem = 3023

| EC_number = 205-072-9

}}

| Section2 = {{Chembox Properties

| Formula = C12H8S

| MolarMass = 184.26 g/mol

| Appearance = Colourless crystals

| Density = 1.252 g/cm3

| Solubility = insol.

| Solvent = other solvents

| SolubleOther = benzene and related

| MeltingPtC = 97 to 100

| MeltingPt_notes = (lit.)

| BoilingPtC = 332 to 333

| BoilingPt_notes =

| pKb =

}}

| Section3 = {{Chembox Structure

| CrystalStruct =

| Dipole =

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| Section7 = {{Chembox Hazards

| ExternalSDS =

| MainHazards = flammable, toxic

| FlashPt =

| GHSPictograms = {{GHS skull and crossbones}}{{GHS exclamation mark}}{{GHS environment}}

| GHSSignalWord = Danger

| HPhrases = {{H-phrases|301|302|311|315|331|332|410}}

| PPhrases = {{P-phrases|261|264|270|271|273|280|301+312|302+352|304+312|304+340|311|312|321|322|330|332+313|361|362|363|391|403+233|405|501}}

}}

| Section8 = {{Chembox Related

| OtherCompounds = Thiophene
Anthracene
Benzothiophene
Dibenzofuran

}}

}}

Dibenzothiophene (DBT, diphenylene sulfide) is the organosulfur compound consisting of two benzene rings fused to a central thiophene ring. It has the chemical formula C12H8S. It is a colourless solid that is chemically somewhat similar to anthracene. This tricyclic heterocycle, and especially its disubstituted derivative 4,6-dimethyldibenzothiophene are problematic impurities in petroleum.{{cite journal|doi=10.1016/j.cattod.2004.07.048|title=Deep HDS of Diesel Fuel: Chemistry and Catalysis |year=2004 |last1=Ho |first1=Teh C. |journal=Catalysis Today |volume=98 |issue=1–2 |pages=3–18 }}

Synthesis and reactions

Dibenzothiophene is prepared by the reaction of biphenyl with sulfur dichloride in the presence of aluminium chloride.{{cite journal|doi=10.1002/jhet.5570150407|title=The Insertion and Extrusion of Heterosulfur Bridges. VIII. Dibenzothiophene from Biphenyl and Derivatives |year=1978 |last1=Klemm |first1=L. H. |last2=Karchesy |first2=Joseph J. |journal=Journal of Heterocyclic Chemistry |volume=15 |issue=4 |pages=561–563 }}

Reduction with lithium results in scission of one C-S bond. With butyllithium, this heterocycle undergoes stepwise lithiation at the 4-position. S-oxidation with peroxides gives the sulfoxide.{{cite journal |doi=10.15227/orgsyn.096.0258|title=Preparation of 5-(Triisopropylalkynyl) dibenzo[b,d]thiophenium triflate |year=2019 |last1=Waldecker |first1=Bernd |journal=Organic Syntheses |volume=96 |pages=258–276 |s2cid=239319277|first2= Kevin|last2=Kafuta|first3=Manuel|last3=Alcarazo|doi-access=free }}

Dibenzothiophene is electron-rich, and naturally undergoes aromatic substitution para to the sulfide. Oxidation to the sulfoxide or sulfone leaves the compound electron poor, and substitution occurs at the meta position instead.{{cite encyclopedia|title=Encyclopedia of Reagents for Organic Synthesis|doi=10.1002/047084289X.rn02046|entry=Dibenzothiophene 5,5-dioxide|first1=M.|last1=Bhanuchandra|author2=Yorimitsu Hideki}}

References