:Dimethylphosphine oxide

{{Chembox

| ImageFile = Me2P(O)H.png

| ImageSize =

| ImageAlt =

| PIN = Dimethyl-λ5-phosphanone

| OtherNames = dimethylphosphinous acid tautomer

|Section1={{Chembox Identifiers

| CASNo = 7211-39-4

| PubChem = 81631

| ChemSpiderID = 10415346

| EC_number = 230-591-2

| SMILES = CP(=O)C

| StdInChI = 1S/C2H7OP/c1-4(2)3/h4H,1-2H3

| StdInChIKey = HGDIHUZVQPKSMO-UHFFFAOYSA-N}}

|Section2={{Chembox Properties

|C = 2|H = 7|O = 1|P = 1

| MolarMass =

| Appearance = colorless liquid

| Density =

| MeltingPt =

| BoilingPt = 65–67 °C

| Solubility = }}

|Section3={{Chembox Hazards

| GHSPictograms = {{GHS07}}

| GHSSignalWord = Warning

| HPhrases = {{H-phrases|302|315|319|335}}

| PPhrases = {{P-phrases|261|264|270|271|280|301+312|302+352|304+340|305+351+338|312|321|330|332+313|337+313|362|403+233|405|501}}

| MainHazards =

| FlashPt =

| AutoignitionPt = }}

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Dimethylphosphine oxide is an organophosphorus compound with the formula (CH3)2P(O)H. It is a colorless liquid that soluble in polar organic solvents. It exists as the phosphine oxide, not the hydroxy tautomer. A related compound is diphenylphosphine oxide. Both are sometimes called secondary phosphine oxides.

Preparation

The compound arises by the hydrolysis of chlorodimethylphosphine:{{cite journal|author=Kleiner, H. J.|title=Herstellung und Umsetzungen von Dimethylphosphinoxid (Preparation and Reactions of Dimethylphosphine Oxide)|journal=Justus Liebigs Ann. Chem.|year=1974|pages=751-764|doi=10.1002/jlac.197419740507}}

:Me2PCl + H2O → Me2P(O)H + HCl

Methanol, but not ethanol, can also be used in place of water, the co-product being methyl chloride.

Since chlorodimethylphosphine is dangerous to handle, alternative routes to dimethylphosphine oxide have been developed. A popular method starts with diethylphosphite, according to the following idealized equations:{{cite journal|author=Hays, H. R.|title=Reaction of diethyl phosphonate with methyl and ethyl Grignard reagents|journal=J. Org. Chem.|year=1968|volume=33|pages=3690-3694|doi=10.1021/jo01274a003}}

:(C2H5O)2P(O)H + 3 CH3MgBr → (CH3)2P(O)MgBr + 2 MgBr(OC2H5) + CH4

:(CH3)2P(O)MgBr + H2O → (CH3)2P(O)H + 2 MgBr(OH)

Reactions

Chlorination gives dimethylphosphoryl chloride. It undergoes hydroxymethylation with formaldehyde.

:Me2P(O)H + CH2O → Me2P(O)CH2OH

Many aldehydes effect a similar reaction.

References