Asx turn

{{Short description|Feature in proteins and polypeptides}}

The Asx turn{{cite book|last=Richardson|first=JS|chapter=The anatomy and taxonomy of protein structure|year=1981|volume=34|pages=167–339 |pmid=7020376|doi=10.1016/S0065-3233(08)60520-3|isbn=9780120342341|title=Advances in Protein Chemistry Volume 34}}{{cite journal|last=Tainer|first=JA|author2=Getzoff ED|authorlink2=Elizabeth D. Getzoff|title=Determination and analysis of the 2 A-structure of copper, zinc superoxide dismutase|journal=Journal of Molecular Biology|year=1982|volume=160|pages=181–217 |pmid=7175933 |doi=10.1016/0022-2836(82)90174-7|issue=2}}{{cite journal|last=Rees|first=DC|author2=Lewis M|title=Refined crystal structure of carboxypeptidase a at 1.54 Å resolution|journal=Journal of Molecular Biology|year=1983|volume=168|pages=367–387 |pmid=6887246|doi=10.1016/S0022-2836(83)80024-2|issue=2}}{{cite journal|last=Eswar|first=N|author2=Ramachandran C|title=Secondary structures without backbone: An analysis of backbone mimicry by polar side chains in proteins|journal=Protein Engineering|year=1999|volume=12|issue=6|pages=447–455|doi=10.1093/protein/12.6.447|pmid=10388841|doi-access=free}}{{cite journal|last=Chakrabarti|first=P|author2=Pal D|title=Interrelationships of side-chain and main-chain conformations in proteins|journal=Progress in Biophysics and Molecular Biology|year=2001|volume=76|issue=1–2|pages=1–102|doi=10.1016/s0079-6107(01)00005-0|pmid=11389934|doi-access=free}}{{cite journal|last=Duddy|first=WJ|author2=Nissink WMJ|title=Mimicry by asx- and ST-turns of the four main types of β-turn in proteins|journal=Protein Science|year=2004|volume=13|issue=11|pages=3051–3055|doi=10.1110/ps.04920904|pmid=15459339|last3=Allen|first3=Frank H.|last4=Milner-White|first4=E. James|pmc=2286581}}{{cite journal|last=Thakur|first=AK|author2=Kishore R|title=Characterization of β-turn and asx-turns mimicry in a model peptide : Stabilization via C-H•••O interaction|journal=Biopolymers|year=2006|volume=81|issue=6|pages=440–449|doi=10.1002/bip.20441|pmid=16411188|s2cid=27091571 }}

is a structural feature in proteins and polypeptides. It consists of three amino acid residues (labeled i, i+1 and i+2) in which residue i is an aspartate (Asp) or asparagine (Asn) that forms a hydrogen bond from its sidechain CO group to the mainchain NH group of residue i+2. About 14% of Asx residues present in proteins belong to Asx turns.

The name "Asx" is used here to represent either of the amino acids aspartate (Asp) or asparagine (Asn).

Types

File:Figure of asx-turn.png

Four types of Asx turn can be distinguished:{{cite journal|last=Duddy|first=WJ|author2=Nissink WMJ|title=Mimicry by asx- and ST-turns of the four main types of beta turn in proteins|journal=Protein Science|year=2004|volume=13|issue=11|pages=3051–3055|doi=10.1110/ps.04920904|pmid=15459339|last3=Allen|first3=Frank H.|last4=Milner-White|first4=E. James|pmc=2286581}} types I, I’, II and II’. These categories correspond to those of the better-known hydrogen-bonded beta turns, which have four residues and a hydrogen bond between the CO of residue i and the NH of residue i+3. Asx turns and beta turns have structurally similar hydrogen-bonded loops and exhibit sidechain-mainchain mimicry in the sense that the sidechain of residue i of the Asx turn mimics the mainchain of residue i of the beta turn. Regarding their occurrence in proteins, they differ in that type I is the commonest of the four beta turns while type II’ is the commonest of the Asx turns.

Occurrence

Asx and ST turns both occur frequently at the N-termini of α-helices.{{cite journal|last=Doig|first=AJ|author2=Macarthur MW|title=Structures of N-termini of helices in proteins|journal=Protein Science|year=1997|volume=6|issue=1|pages=147–155|doi=10.1002/pro.5560060117|pmid=9007987|pmc=2143508|last3=MacArthur|first3=Malcolm W.|last4=Thornton|first4=Janet M.}}{{cite journal|last=Presta|first=LG|author2=Rose GD |title=Helix Caps|journal=Science|year=1988|volume=240|issue=4859|pages=1632–1641|doi= 10.1126/science.2837824|pmid=2837824|bibcode=1988Sci...240.1632P}}{{cite journal|last=Aurora|first=R|author2=Rose GD |title=Helix Capping|journal=Protein Science|year=1998|volume=7|issue=1|pages=21–38|doi= 10.1002/pro.5560070103|pmid=9514257|pmc=2143812}}{{cite journal|last=Gunasekaran|first=K|author2=Nagarajam HA |title=Stereochemical punctuation marks in protein structure|journal=Journal of Molecular Biology|year=1998|volume=275|issue=5|pages=917–932|doi= 10.1006/jmbi.1997.1505|pmid=9480777|last3=Ramakrishnan|first3=C|last4=Balaram|first4=P|s2cid=35919397}} as part of Asx motifs or ST motifs such that the Asx, serine or threonine is the N cap residue. They are thus often regarded as helix capping features.

Related motifs

Similar motifs occur with serine or threonine as residue i, which are called ST turns.{{cite journal|last=Duddy|first=WJ|author2=Nissink WMJ|title=Mimicry by asx- and ST-turns of the four main types of β-turn in proteins|journal=Protein Science|year=2004|volume=13|issue=11|pages=3051–3055|doi=10.1110/ps.04920904|pmid=15459339|last3=Allen|first3=Frank H.|last4=Milner-White|first4=E. James|pmc=2286581}} In spite of serine and threonine having one less sidechain atom, such that the sidechain-mainchain mimicry of β turns is imperfect, these features occur in proteins as the four types in numbers approaching those of Asx turns. They also exhibit a tendency to substitute each other over evolutionary time.{{cite journal|last=Wan|first=W-Y|author2=Milner-White EJ|title=A Recurring Two-Hydrogen-bond Motif Incorporating a Serine or Threonine Residue is found both at α-Helical N Termini and in Other Situations|journal=Journal of Molecular Biology|year=2009|volume=286|issue=5|pages=1651–1662|doi=10.1006/jmbi.1999.2551|pmid=10064721}}

A proportion of Asx turns are accompanied by a mainchain–mainchain hydrogen bond that qualifies them as Asx motifs.

References