Dextrorphan

{{Short description|Psychoactive cough suppressant medication}}

{{Distinguish|Dextromethorphan|Dextrallorphan}}

{{Infobox drug

| Verifiedfields = changed

| Watchedfields = changed

| verifiedrevid = 408496712

| IUPAC_name = (+)-17-methyl-9a,13a,14a-morphinan-3-ol

| image = Dextrorphan.svg

| image_class = skin-invert-image

| image2 = Dextrorphane 3d.gif

| tradename =

| legal_US = Unscheduled{{Cite web |last=Bensinger |first=Peter |date=October 1, 1976 |title=Dextrophan and Nalbuphine; Removal from Schedules |url=https://www.govinfo.gov/content/pkg/FR-1976-10-01/pdf/FR-1976-10-01.pdf |access-date=June 26, 2023 |website=NARA}}

| CAS_number_Ref = {{cascite|correct|??}}

| CAS_number = 125-73-5

| ATC_prefix = None

| PubChem = 5360697

| UNII_Ref = {{fdacite|changed|FDA}}

| UNII = 04B7QNO9WS

| ChEMBL_Ref = {{ebicite|changed|EBI}}

| ChEMBL = 1254766

| ChemSpiderID_Ref = {{chemspidercite|changed|chemspider}}

| ChemSpiderID = 10489895

| synonyms = DXO, Dextrorphanol

| C = 17

| H = 23

| N = 1

| O = 1

| SMILES = CN1CC[C@@]23CCCC[C@@H]2[C@@H]1Cc4c3cc(O)cc4

| StdInChI_Ref = {{stdinchicite|changed|chemspider}}

| StdInChI = 1S/C17H23NO/c1-18-9-8-17-7-3-2-4-14(17)16(18)10-12-5-6-13(19)11-15(12)17/h5-6,11,14,16,19H,2-4,7-10H2,1H3/t14-,16+,17+/m1/s1

| StdInChIKey_Ref = {{stdinchicite|changed|chemspider}}

| StdInChIKey = JAQUASYNZVUNQP-PVAVHDDUSA-N

}}

Dextrorphan (DXO) is a psychoactive drug of the morphinan class which acts as an antitussive or cough suppressant and in high doses a dissociative hallucinogen. It is the dextrorotatory enantiomer of racemorphan; the levorotatory enantiomer is levorphanol. Dextrorphan is produced by O-demethylation of dextromethorphan by CYP2D6. Dextrorphan is an NMDA antagonist and contributes to the psychoactive effects of dextromethorphan.{{cite journal | vauthors = Zawertailo LA, Kaplan HL, Busto UE, Tyndale RF, Sellers EM | title = Psychotropic effects of dextromethorphan are altered by the CYP2D6 polymorphism: a pilot study | journal = Journal of Clinical Psychopharmacology | volume = 18 | issue = 4 | pages = 332–337 | date = August 1998 | pmid = 9690700 | doi = 10.1097/00004714-199808000-00014 }}

Pharmacology

=Pharmacodynamics=

class="wikitable floatleft" style="font-size:small;"

|+ Dextrorphan{{cite web | title = PDSP Ki Database | work = Psychoactive Drug Screening Program (PDSP)|author1-link=Bryan Roth| vauthors = Roth BL, Driscol J | publisher = University of North Carolina at Chapel Hill and the United States National Institute of Mental Health | access-date = 14 August 2017 | url = https://pdsp.unc.edu/databases/pdsp.php?knowID=0&kiKey=&receptorDD=&receptor=&speciesDD=&species=&sourcesDD=&source=&hotLigandDD=&hotLigand=&testLigandDD=&testFreeRadio=testFreeRadio&testLigand=dextrorphan&referenceDD=&reference=&KiGreater=&KiLess=&kiAllRadio=all&doQuery=Submit+Query}}{{cite journal | vauthors = Nguyen L, Thomas KL, Lucke-Wold BP, Cavendish JZ, Crowe MS, Matsumoto RR | title = Dextromethorphan: An update on its utility for neurological and neuropsychiatric disorders | journal = Pharmacol. Ther. | volume = 159 | pages = 1–22 | year = 2016 | pmid = 26826604 | doi = 10.1016/j.pharmthera.2016.01.016 }}{{cite journal | vauthors = Werling LL, Keller A, Frank JG, Nuwayhid SJ | title = A comparison of the binding profiles of dextromethorphan, memantine, fluoxetine and amitriptyline: treatment of involuntary emotional expression disorder | journal = Exp. Neurol. | volume = 207 | issue = 2 | pages = 248–57 | year = 2007 | pmid = 17689532 | doi = 10.1016/j.expneurol.2007.06.013 | s2cid = 38476281 }}{{cite journal | vauthors = Taylor CP, Traynelis SF, Siffert J, Pope LE, Matsumoto RR | title = Pharmacology of dextromethorphan: Relevance to dextromethorphan/quinidine (Nuedexta®) clinical use | journal = Pharmacol. Ther. | volume = 164 | pages = 170–82 | year = 2016 | pmid = 27139517 | doi = 10.1016/j.pharmthera.2016.04.010 | doi-access = free }}

SiteKi (nM)SpeciesRef
NMDA receptor486–906Rat
σ1118–481Rat
σ211,325–15,582Rat
{{abbrlink|MOR|μ-Opioid receptor}}420
>1,000
Rat
Human
{{cite journal | vauthors = Raynor K, Kong H, Mestek A, Bye LS, Tian M, Liu J, Yu L, Reisine T | title = Characterization of the cloned human mu opioid receptor | journal = J. Pharmacol. Exp. Ther. | volume = 272 | issue = 1 | pages = 423–8 | year = 1995 | pmid = 7815359 }}
{{abbrlink|DOR|δ-Opioid receptor}}34,700Rat
{{abbrlink|KOR|κ-Opioid receptor}}5,950Rat
{{abbrlink|SERT|Serotonin transporter}}401–484Rat
{{abbrlink|NET|Norepinephrine transporter}}≥340Rat
{{abbrlink|DAT|Dopamine transporter}}>1,000Rat
5-HT1A>1,000Rat
5-HT1B/1D54% at 1 μMRat
5-HT2A>1,000Rat
α1>1,000Rat
α2>1,000Rat
β35% at 1 μMRat
D2>1,000Rat
H195% at 1 μMRat
{{abbrlink|mAChRs|Muscarinic acetylcholine receptors}}100% at 1 μMRat
{{abbrlink|nAChRs|Nicotinic acetylcholine receptors}}1,300–29,600
(IC50)
Rat
{{abbrlink|VDSCs|Voltage-dependent sodium channels}}{{abbr|ND|No data}}{{abbr|ND|No data}}{{abbr|ND|No data}}
class="sortbottom"

| colspan="4" style="width: 1px;" | Values are Ki (nM), unless otherwise noted. The smaller the value, the more strongly the drug binds to the site.

The pharmacology of dextrorphan is similar to that of dextromethorphan (DXM). However, dextrorphan is much more potent as an NMDA receptor antagonist and much less active as a serotonin reuptake inhibitor, but retains DXM's activity as a norepinephrine reuptake inhibitor.{{cite journal | vauthors = Pechnick RN, Poland RE | title = Comparison of the effects of dextromethorphan, dextrorphan, and levorphanol on the hypothalamo-pituitary-adrenal axis | journal = The Journal of Pharmacology and Experimental Therapeutics | volume = 309 | issue = 2 | pages = 515–522 | date = May 2004 | pmid = 14742749 | doi = 10.1124/jpet.103.060038 | s2cid = 274504 }}

It also has more affinity for the opioid receptors than dextromethorphan, significantly so at high doses.

=Pharmacokinetics=

Dextrorphan has a notably longer elimination half-life than its parent compound, and therefore has a tendency to accumulate in the blood after repeated administration of normally dosed dextromethorphan formulations.{{citation needed|date=November 2016}} It is further converted to 3-HM by CYP3A4 or glucuronidated.{{cite journal | vauthors = Yu A, Haining RL | title = Comparative contribution to dextromethorphan metabolism by cytochrome P450 isoforms in vitro: can dextromethorphan be used as a dual probe for both CTP2D6 and CYP3A activities? | journal = Drug Metabolism and Disposition | volume = 29 | issue = 11 | pages = 1514–20 | date = November 2001 | pmid = 11602530 | url = http://dmd.aspetjournals.org/cgi/pmidlookup?view=long&pmid=11602530 }}

Society and culture

=Legal status=

Dextrorphan was formerly a Schedule I controlled substance in the United States, but was unscheduled on October 1, 1976.{{cite web | url = http://www.deadiversion.usdoj.gov/schedules/orangebook/orangebook.pdf | title = Lists of: Scheduling Actions Controlled Substances Regulated Chemicals | author = DEA | access-date = 2010-09-24 | archive-date = 2016-04-17 | archive-url = https://web.archive.org/web/20160417085648/http://www.deadiversion.usdoj.gov/schedules/orangebook/orangebook.pdf | url-status = dead }}

Research

Dextrorphan was under development for the treatment of stroke, and reached phase II clinical trials for this indication, but development was discontinued.{{Cite web|url=http://adisinsight.springer.com/drugs/800009336|title = Dextrorphan - AdisInsight}}

Environmental presence

In 2021, dextrorphan was identified in >75% of sludge samples taken from 12 wastewater treatment plants in California. The same study associated dextrorphan with estrogenic activity by using predictive modelling, before observing it in in vitro.{{cite journal | vauthors = Black GP, He G, Denison MS, Young TM | title = Using Estrogenic Activity and Nontargeted Chemical Analysis to Identify Contaminants in Sewage Sludge | journal = Environmental Science & Technology | volume = 55 | issue = 10 | pages = 6729–6739 | date = May 2021 | pmid = 33909413 | pmc = 8378343 | doi = 10.1021/acs.est.0c07846 | bibcode = 2021EnST...55.6729B }}

{{Clear}}

See also

References

{{Reflist|2}}

{{Antitussives}}

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Category:Antitussives

Category:Dissociative drugs

Category:Enantiopure drugs

Category:Euphoriants

Category:Morphinans

Category:Mu-opioid receptor agonists

Category:Nicotinic antagonists

Category:NMDA receptor antagonists

Category:Hydroxyarenes

Category:Serotonin–norepinephrine reuptake inhibitors

Category:Sigma agonists

Category:Human drug metabolites