Ferrocenium tetrafluoroborate

{{chembox

| Watchedfields = changed

| verifiedrevid = 429060751

| ImageFile1 = Ferrocenium_tetrafluoroborate.svg

| ImageFile2 = Ferrocenium-tetrafluoroborate-3D-vdW.png

| ImageFile3 = FcBF4.jpg

| IUPACName = Ferrocenium tetrafluoroborate

|Section1={{Chembox Identifiers

| CASNo_Ref = {{cascite|correct|??}}

| CASNo = 1282-37-7

| EINECS = 627-836-4

| PubChem = 124204127

| PubChem_Comment = charge error

| ChemSpiderID = 69007671

| SMILES = C1=C[CH-]C=C1.[Fe+3].C2=C[CH-]C=C2.F[B-](F)(F)F

| InChI =

}}

|Section2={{Chembox Properties

| Formula = C10H10BFeF4

| MolarMass = 272.84 g/mol

| Appearance = dark blue powder

| Density =

| MeltingPtC = 178

| MeltingPt_notes = (decomposes)

| BoilingPt =

| Solubility =

| SolubleOther = Soluble{{cn|date=January 2013}}

| Solvent = acetonitrile

}}

|Section3={{Chembox Hazards

| Hazards_ref = {{cite web |title=Ferrocenium tetrafluoroborate 482358 |url=https://www.sigmaaldrich.com/catalog/product/aldrich/482358 |website=Sigma-Aldrich}}

| GHSPictograms = {{GHS05}}

| GHSSignalWord = Danger

| HPhrases = {{H-phrases|314}}

| PPhrases = {{P-phrases|280|305+351+338|310 }}

| ExternalSDS = [http://msds.chem.ox.ac.uk/FE/ferrocenium_tetrafluoroborate.html External MSDS]

| FlashPt =

| AutoignitionPt =

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|Section8={{Chembox Related

| OtherCompounds = Ferrocene}}

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Ferrocenium tetrafluoroborate is an organometallic compound with the formula [Fe(C5H5)2]BF4. This salt is composed of the cation [Fe(C5H5)2]+ and the tetrafluoroborate anion ({{chem|BF|4|−}}). The related hexafluorophosphate is also a popular reagent with similar properties. The ferrocenium cation is often abbreviated Fc+ or Cp2Fe+. The salt is deep blue in color and paramagnetic.

Ferrocenium salts are sometimes used as one-electron oxidizing agents, and the reduced product, ferrocene, is inert and readily separated from ionic products. The ferrocene–ferrocenium couple is often used as a reference in electrochemistry. The standard potential of ferrocene-ferrocenium is dependent on specific electrochemical conditions.

Preparation

Commercially available, this compound may be prepared by oxidizing ferrocene typically with ferric salts followed by addition of fluoroboric acid.{{cite journal|first1=N. G.|last1= Connelly|first2= W. E.|last2= Geiger| title=Chemical Redox Agents for Organometallic Chemistry|journal=Chemical Reviews|year= 1996| volume= 96|issue=2| pages= 877–910| doi=10.1021/cr940053x| pmid=11848774}} A variety of other oxidants work well also, such as nitrosyl tetrafluoroborate.{{cite journal | title = Solvent and electrolyte effects on the kinetics of ferrocenium-ferrocene self-exchange. A reevaluation | first1= Roger M.|last1= Nielson|first2= George E.|last2= McManis|first3= Lance K.|last3= Safford|first4= Michael J. |last4=Weaver | journal = J. Phys. Chem. | doi = 10.1021/j100342a086 | year = 1989 | volume = 93 | issue = 5 | pages = 2152}} Many analogous ferrocenium salts are known.{{cite journal|first1=J.|last1= Le Bras|first2= H. |last2=Jiao |first3=W. E. |last3=Meyer |first4=F.|last4= Hampel |first5= J. A.|last5= Gladysz |title=Synthesis, Crystal Structure, and Reactions of the 17-Valence-Electron Rhenium Methyl Complex [(η5-C5Me5)Re(NO)(P(4-C6H4CH3)3)(CH3)]+ {{chem|B(3,5-C|6|H|3|(CF|3|)|2|)|4|−}}: Experimental and Computational Bonding Comparisons with 18-Electron Methyl and Methylidene Complexes |journal=J. Organomet. Chem.|date= 2000 |volume= 616 |pages= 54–66 |doi=10.1016/S0022-328X(00)00531-3}}

Structure

According to X-ray crystallography, the structures of the metallocene component of FcBF4 and the parent ferrocene are very similar. The Fe-C distances in the cation are 209.5 pm, about 2% longer than the Fe-C distances in ferrocene.

{{cite journal |doi=10.1016/j.ica.2007.03.049 |title=Difference in Reactivity of Triel Halides EX3 Towards Ferrocene |date=2007 |last1=Scholz |first1=Stefan |last2=Scheibitz |first2=Matthias |last3=Schödel |first3=Frauke |last4=Bolte |first4=Michael |last5=Wagner |first5=Matthias |last6=Lerner |first6=Hans-Wolfram |journal=Inorganica Chimica Acta |volume=360 |issue=10 |pages=3323–3329 }}

References

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{{iron compounds}}

{{Tetrafluoroborates}}

Category:Ferrocenes

Category:Tetrafluoroborates

Category:Oxidizing agents